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Transition Metal Carbonitride MXenes Anchored with Pt Sub-Nanometer Clusters to Achieve High-Performance Hydrogen Evolution Reaction at All pH Range

Authors: Zhihao Lei; Sajjad Ali; CI Sathish; Muhammad Ibrar Ahmed; Jiangtao Qu; Rongkun Zheng; Shibo Xi; Xiaojiang Yu; M. B. H. Breese; Chao Liu; Jizhen Zhang; Shuai Qi; Xinwei Guan; Vibin Perumalsamy; Mohammed Fawaz; Jae-Hun Yang; Mohamed Bououdina; Kazunari Domen; Ajayan Vinu; Liang Qiao; Jiabao Yi

DOI: 10.1007/s40820-025-01654-yStatus: Verified Translated Edition

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Key Findings in This Report

• Two-dimensional mono- and few-layered Ti3CNTx MXene nanosheets with extremely high nitrogen content were synthesized. • Better performance for hydrogen evolution reaction (HER) than Pt/C catalyst in acidic, neutral and alkaline solutions. • Exceptional performance of HER in both acidic and alkaline solutions. • A large current density (>500 mA cm−2) has been achieved for HER.