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Scalable Electrocatalytic Urea Wastewater Treatment Coupled with Hydrogen Production by Regulating Adsorption Behavior of Urea Molecule

Authors: Chunming Yang; Huijuan Pang; Xiang Li; Xueyan Zheng; Tingting Wei; Xu Ma; Qi Wang; Chuantao Wang; Danjun Wang; Bin Xu

DOI: 10.1007/s40820-024-01585-0Status: Verified Translated Edition
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Key Findings in This Report

• The heterogeneous interface of NiO/Co3O4 regulates urea adsorption behavior, enhancing UOR kinetics. • DFT and TPD experiments confirm the mechanism of charge redistribution and functional group adsorption. • AEMWE with NiO/Co3O4 anode and NiCoP cathode achieves scalable urea wastewater treatment at 600 mA cm−2 with ~53% efficiency. • Hydrogen production rate is 3.5 times higher than overall water splitting, offering energy-saving and cost-effective wastewater treatment.
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