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Porous Microreactor Chip for Photocatalytic Seawater Splitting over 300 Hours at Atmospheric Pressure

Authors: Desheng Zhu; Zhipeng Dong; Chengmei Zhong; Junhong Zhang; Qi Chen; Ni Yin; Wencheng Jia; Xiong Zheng; Fengzai Lv; Zhong Chen; Zhenchao Dong; Wencai Huang

DOI: 10.1007/s40820-025-01703-6Status: Verified Translated Edition
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Key Findings in This Report

• A film-type Ag3PO4/CdS photocatalyst in a porous substrate configuration is designed and prepared to avoid photocorrosion and ensure outstanding firmness. • Both the S and Ag vacancy-rich surface and the heterojunction within the space charge region are found to be the key for high solar-to-hydrogen efficiency and excellent stability in seawater over 300 h. • The first fully solar-driven hydrogen production prototype is constructed to work outdoors, exhibiting a high H2 evolution rate of 68.01 mmol h−1 m−2. • The separation of oxidation and reduction reactions in space inhibits reverse recombination, enabling operation at atmospheric pressure and scalable practical solar H2 production.