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An Ultra-Stable, High-Energy and Wide-Temperature-Range Aqueous Alkaline Sodium-Ion Battery with the Microporous C4N/rGO Anode

Authors: Mengxiao Li; Rui Li; Huige Ma; Mingsheng Yang; Yujie Dai; HaiPing Yu; Yuxin Hao; Zhihui Wang; Bei Wang; Mingjun Hu; Jun Yang

DOI: 10.1007/s40820-024-01589-wStatus: Verified Translated Edition
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Key Findings in This Report

• An integrated conjugated microporous polymer composite electrode (C4N/rGO) with high conductivity, large specific surface area and good solvent resistance was prepared by in-situ growth. • An antifreeze alkaline electrolyte (0.1 DMSO/2 M NaOH) was developed to broaden the operation temperature zone and voltage window of the aqueous alkaline battery. • The prepared aqueous alkaline battery exhibits a high energy density (147.3 Wh Kg−1 at 25 °C), outstanding long cycling stability and excellent wide-temperature-range performance (−70 to 45 °C). • The C4N/rGO//Ni(OH)2 full cell demonstrates ultra-high cycling stability over 38,000 cycles, offering a promising solution for extreme-condition energy storage.