• A novel LM/CIP/PDMS composite with core-shell structure combines magnetic and dielectric properties for enhanced EMW absorption.
• The addition of EGaIn liquid metal improves mechanical flexibility and introduces dielectric loss mechanisms, overcoming the limitations of pure magnetic CIP fillers.
• Mechanical strain induces the formation of a conductive LM network, further enhancing EMW absorption performance.
• The composite offers a promising solution for flexible, stretchable EMW-absorbing materials to mitigate electromagnetic pollution in advanced wireless technologies.
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