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Realizing stable zinc anodes via three-dimensional passivation layer

Authors: Shi LI; Xin-wei DAI; Rui-bo JIANG; Yan-ting CAI; Lan-yan LI; Zhong-min WAN; Xi CHEN; Xiang-zhong KONG; Guo-zhao FANG

DOI: 10.1016/S1003-6326(25)67030-0Status: Verified Translated Edition
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Key Findings in This Report

• A porous 3D structure on Zn surface via electrostripping activation suppresses non-uniform Zn2+ deposition and dendrite growth. • A functional CeO4H4/Ce(OH)3 passivation layer prevents electrochemical corrosion and enhances electrolyte infiltration. • The symmetric cell achieves over 1500 h lifespan at 5 mA/cm2 and over 300 h at 20 mA/cm2. • The R-Zn@CeǁMnO2 full cell delivers a capacity of 205.3 mA·h/g after 300 cycles at 0.3 A/g.