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Kinetics and morphological evolution mechanism of WO3 during non-isothermal hydrogen reduction

Authors: Rui-fang WANG; Xiang ZHAN; Yong-qiang CHEN; Shi-ming ZHANG; Yu-si CHE; Ji-lin HE

DOI: 10.1016/S1003-6326(25)66986-XStatus: Verified Translated Edition
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Key Findings in This Report

• Non-isothermal thermogravimetric analysis reveals two-stage hydrogen reduction kinetics of WO3 with activation energies of 121 and 135 kJ/mol for the first and second stages, respectively. • Under local gas–solid reduction conditions, the particle morphology of tungsten powders mirrors that of the raw WO3, with porous structures forming between reduced particles. • The porous morphology of reduced tungsten powders contrasts with the polyhedral single-crystal configuration obtained via chemical vapor deposition. • The two-stage hydrogen reduction mechanisms of WO3 can be accurately described using a composite autocatalytic function.