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Hydrogel Electrolytes for Zinc-Ion Batteries: Materials Design, Functional Strategies, and Future Perspectives

Authors: Zhengchu Zhang; Yongbiao Mu; Lijuan Xiao; Hengyuan Hu; Tao Xue; Limin Zang; Eiichi Sakai; Meisheng Han; Chao Yang; Lin Zeng; Jianhui Qiu

DOI: 10.1007/s40820-025-01993-wStatus: Verified Translated Edition
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Key Findings in This Report

• Hydrogel electrolytes combine high ionic conductivity with mechanical robustness, effectively suppressing zinc dendrite growth and enhancing interfacial stability in zinc-ion batteries. • Design strategies encompass natural polymers, synthetic polymers, and composites, with tunable properties via electrolyte salts and functional additives. • Functional optimizations include anti-freezing, self-healing, thermal responsiveness, and biocompatibility, enabling operation under extreme conditions. • Future development focuses on green, safe, and multifunctional integrated optimization to overcome current challenges.
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