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Hydrogel Electrolytes-Based Rechargeable Zinc-Ion Batteries under Harsh Conditions

Authors: Zhaoxi Shen; Zicheng Zhai; Yu Liu; Xuewei Bao; Yuechong Zhu; Tong Zhang; Linsen Li; Guo Hong; Ning Zhang

DOI: 10.1007/s40820-025-01727-yStatus: Verified Translated Edition
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Key Findings in This Report

• Hydrogel electrolytes effectively address limitations of aqueous electrolytes in zinc-ion batteries, including dendrite growth, side reactions, and cathode dissolution. • Functional designs of hydrogel electrolytes enable operation under harsh conditions: extreme temperatures, mechanical deformations, and physical damages. • The review systematically covers fundamentals, species, and mechanisms of hydrogel electrolytes, along with their compatibility with Zn anodes and cathodes. • Future perspectives highlight remaining challenges and opportunities for practical application of hydrogel electrolyte-based rechargeable zinc-ion batteries.