• A novel reinforcement fluid that undergoes liquid-gas phase transition in vacuum is proposed for lunar borehole stabilization.
• The developed reinforcement liquid increases the cohesion of simulated lunar soil from 2 to 800 kPa, significantly enhancing borehole stability.
• High-vacuum (5 Pa) and low-temperature (−30 to 50 °C) coring experiments confirm spontaneous release and effective borehole reinforcement.
• Optimal solute concentration for borehole reinforcement is between 0.15 and 0.25 g/mL.
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